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POSTSUBSCRIPT ∼ 105 K which can not be described by a Curie-Weiss legislation. POSTSUBSCRIPT symmetry might be clearly identified. In crossed polarization magnetic excitations of different symmetry can contribute to the Raman sign. POSTSUBSCRIPT, which is detected in our Raman spectra, points to such a possibility. POSTSUBSCRIPT, the compound undergoes a magnetic section transition into a long-vary-ordered state. 25 K. Here, an exterior magnetic discipline leads to a transition from an AFM to a ferrimagnetic state. The particular ratio of the saw-tooth spine-spine and spine-vertex interactions may clarify the instability of the dimer quantum ground state towards an incommensurate 3D magnetic order. The LSW theory can capture an incommensurate instability of the given 3D uniform lengthy-range order underneath detection of some spin wave approaching zero energy at a sure wave vector. It’s price repeating that this last interplay is liable for establishing lengthy-vary order. It’s additionally a continually shifting target.
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